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New trendy magnetic C-scorpionate iron catalyst and its performance towards cyclohexane oxidation

2018-02Journal article Restricted access
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dc.contributor.authorDa Costa Ribeiro, Ana Paula
dc.contributor.authorMatias, Inês
dc.contributor.authorAlegria, Elisabete
dc.contributor.authorFerraria, Ana Maria
dc.contributor.authorRego, Ana
dc.contributor.authorPombeiro, Armando
dc.contributor.authorMartins, Luisa
dc.date.accessioned2018-04-19T10:49:18Z
dc.date.available2018-04-19T10:49:18Z
dc.date.issued2018-02
dc.description.abstractFor the first time, a magnetic C-scorpionate catalyst was prepared from the iron(II) complex [FeCl2{_3-HC(pz)3}] (pz = pyrazol-1-yl) and ferrite, using the sustainable mechanochemical synthetic procedure. Its catalytic activity for the cyclohexane oxidation with tert-butyl hydroperoxide (TBHP) was evaluated in different conditions, namely under microwave irradiation and under the effect of an external magnetic field. The use of such magnetic conditions significantly shifted the catalyst alcohol/ketone selectivity, thus revealing a promising, easy new protocol for tuning selectivity in important catalytic processes.pt_PT
dc.description.versioninfo:eu-repo/semantics/publishedVersionpt_PT
dc.identifier.citationRIBEIRO, Ana P. C.; [et al] – New trendy magnetic C-scorpionate iron catalyst and its performance towards cyclohexane oxidation. Catalysts. ISSN 2073-4344. Vol. 8, N.º 2 (2018), pp. 1-11pt_PT
dc.identifier.doi10.3390/catal8020069pt_PT
dc.identifier.issn2073-4344
dc.identifier.urihttp://hdl.handle.net/10400.21/8423
dc.language.isoengpt_PT
dc.peerreviewedyespt_PT
dc.publisherMDPIpt_PT
dc.relationSmart biopolymer surfaces for Chemical Warfare Agents catalytic degradation: involved mechanisms
dc.subjectMagneticpt_PT
dc.subjectC-scorpionatept_PT
dc.subjectCatalystpt_PT
dc.subjectOxidationpt_PT
dc.subjectSelectivitypt_PT
dc.subjectMechanochemicalpt_PT
dc.subjectCyclohexanept_PT
dc.subjectIronpt_PT
dc.titleNew trendy magnetic C-scorpionate iron catalyst and its performance towards cyclohexane oxidationpt_PT
dc.typejournal article
dspace.entity.typePublication
oaire.awardTitleSmart biopolymer surfaces for Chemical Warfare Agents catalytic degradation: involved mechanisms
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oaire.citation.endPage11pt_PT
oaire.citation.issue2pt_PT
oaire.citation.startPage1pt_PT
oaire.citation.titleCatalystspt_PT
oaire.citation.volume8pt_PT
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person.familyNameda Costa Ribeiro
person.familyNameMatias
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person.givenNameAna Paula
person.givenNameInês
person.givenNameElisabete
person.givenNameAna Maria
person.givenNameAna
person.givenNameArmando
person.givenNameLuisa
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rcaap.typearticlept_PT
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