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Reentrant Phase Diagram of Network Fluids

2011-02-25Journal article Open access
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dc.contributor.authorRusso, J.
dc.contributor.authorTavares, Jose
dc.contributor.authorTeixeira, Paulo
dc.contributor.authorGama, Margarida
dc.contributor.authorSCIORTINO, Francesco
dc.date.accessioned2013-02-16T18:04:46Z
dc.date.available2013-02-16T18:04:46Z
dc.date.issued2011-02-25
dc.description.abstractWe introduce a microscopic model for particles with dissimilar patches which displays an unconventional "pinched'' phase diagram, similar to the one predicted by Tlusty and Safran in the context of dipolar fluids [Science 290, 1328 (2000)]. The model-based on two types of patch interactions, which account, respectively, for chaining and branching of the self-assembled networks-is studied both numerically via Monte Carlo simulations and theoretically via first-order perturbation theory. The dense phase is rich in junctions, while the less-dense phase is rich in chain ends. The model provides a reference system for a deep understanding of the competition between condensation and self-assembly into equilibrium-polymer chains.en
dc.identifier.citationRUSSO, J.; TAVARES, J. M.; TEIXEIRA, P. I. C.; DA GAMA, M. M. Telo; SCIORTINO, F. - Reentrant Phase Diagram of Network Fluids. Physical Review Letters. ISSN 0031-9007. Vol. 106, n.º 8 (2011).por
dc.identifier.issn0031-9007
dc.identifier.urihttp://hdl.handle.net/10400.21/2234
dc.language.isoengpor
dc.peerreviewedyespor
dc.publisherAmer Physical Socpor
dc.relation.ispartofseries085703
dc.relation.publisherversionhttp://journals.aps.org/prl/abstract/10.1103/PhysRevLett.106.085703
dc.subjectDirectional Attractive Forcespor
dc.subjectDipolar Hard-Spherespor
dc.subjectMonte-Carlopor
dc.subjectThermodynamicspor
dc.subjectParticlespor
dc.subjectSystemspor
dc.subjectPatchypor
dc.titleReentrant Phase Diagram of Network Fluidspor
dc.typejournal article
dspace.entity.typePublication
oaire.citation.conferencePlaceUSApor
oaire.citation.issue8por
oaire.citation.titlePhysical Review Letterspor
oaire.citation.volume106por
person.familyNameTavares
person.familyNameTeixeira
person.familyNameTelo da Gama
person.familyNameSCIORTINO
person.givenNameJose
person.givenNamePaulo
person.givenNameMargarida Maria
person.givenNameFrancesco
person.identifierhttps://scholar.google.pt/citations?user=OrsjRkYAAAAJ&hl=pt-PT
person.identifier.ciencia-id371D-51C6-975C
person.identifier.ciencia-idB31A-0CBD-8AC4
person.identifier.ciencia-idB811-A73C-181F
person.identifier.orcid0000-0002-1509-9707
person.identifier.orcid0000-0003-2315-2261
person.identifier.orcid0000-0002-2418-2713
person.identifier.ridA-2891-2009
person.identifier.ridA-2682-2009
person.identifier.scopus-author-id35621140500
person.identifier.scopus-author-id7005895098
person.identifier.scopus-author-id0000-0001-8849-9990
person.identifier.scopus-author-id7005775345
rcaap.rightsrestrictedAccesspor
rcaap.typearticlepor
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relation.isAuthorOfPublication35a012c6-2e8b-402f-9b82-065843fce9aa
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relation.isAuthorOfPublication.latestForDiscovery4fde2efd-f48f-4419-b383-74945fb2db28

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