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Enhancing alkane oxidation using Co-doped SnO2 nanoparticles as catalysts

2017-06Journal article Restricted access
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dc.contributor.authorSilva, Telma F.S.
dc.contributor.authorSilvestre, A. J.
dc.contributor.authorRocha, Bruno G. M.
dc.contributor.authorNunes, Manuel R.
dc.contributor.authorMonteiro, Olinda
dc.contributor.authorMartins, Luisa
dc.date.accessioned2017-03-28T07:31:37Z
dc.date.available2017-03-28T07:31:37Z
dc.date.issued2017-06
dc.description.abstractA novel eco-friendly KA oil synthesis at room temperature (up to 25% yield) via solvent-free cyclohexane oxidation using Sn1 − xCoxO2 − δ (x = 0, 0.01 or 0.05) nanoparticles as catalyst (TON up to 2 × 103) is here reported. These nanoparticles are the first SnO2-based material able to catalyze the oxidation of alkanes. The most active nanocatalyst was the Sn0.95Co0.05O2 − δ, allowing an easy recovery and reuse, at least for five consecutive cycles, maintaining high selectivity concomitant with 92% of its initial activity.pt_PT
dc.description.versioninfo:eu-repo/semantics/acceptedVersionpt_PT
dc.identifier.citationSILVA, Telma F. S.; [et al] – Enhancing alkane oxidation using Co-doped SnO2 nanoparticles as catalysts. Catalysis Communications. ISSN 1566-7367. Vol. 96 (2017), pp. 19-22.pt_PT
dc.identifier.doihttp://dx.doi.org/10.1016/j.catcom.2017.03.012pt_PT
dc.identifier.issn1566-7367
dc.identifier.urihttp://hdl.handle.net/10400.21/6886
dc.language.isoengpt_PT
dc.peerreviewedyespt_PT
dc.publisherElsevierpt_PT
dc.relation.publisherversionhttp://ac.els-cdn.com/S1566736717300973/1-s2.0-S1566736717300973-main.pdf?_tid=ae5a1fb4-1386-11e7-b7a6-00000aacb361&acdnat=1490685663_6efbc8225d244011b0101a57996640e3pt_PT
dc.subjectAlkanept_PT
dc.subjectSnO2pt_PT
dc.subjectNanoparticlespt_PT
dc.subjectNanocatalystpt_PT
dc.subjectOxidationpt_PT
dc.subjectRecyclept_PT
dc.titleEnhancing alkane oxidation using Co-doped SnO2 nanoparticles as catalystspt_PT
dc.typejournal article
dspace.entity.typePublication
oaire.citation.endPage22pt_PT
oaire.citation.startPage19pt_PT
oaire.citation.titleCatalysis Communicationspt_PT
oaire.citation.volume96pt_PT
person.familyNameSilvestre
person.familyNameRocha
person.familyNameMonteiro
person.familyNameMartins
person.givenNameAntónio Jorge
person.givenNameBruno G. M.
person.givenNameOlinda
person.givenNameLuisa
person.identifier2748637
person.identifier637885
person.identifier.ciencia-id9C18-D57C-7958
person.identifier.ciencia-idDA12-8EB9-8DA3
person.identifier.ciencia-idE218-E297-A4EA
person.identifier.orcid0000-0001-6517-6275
person.identifier.orcid0000-0003-0357-0677
person.identifier.orcid0000-0002-1134-4680
person.identifier.orcid0000-0002-5403-9352
person.identifier.ridG-3614-2017
person.identifier.ridD-9936-2012
person.identifier.ridG-6210-2011
person.identifier.scopus-author-id25224208600
person.identifier.scopus-author-id55179069100
person.identifier.scopus-author-id7006528144
person.identifier.scopus-author-id8650947800
rcaap.rightsrestrictedAccesspt_PT
rcaap.typearticlept_PT
relation.isAuthorOfPublicationda27d795-d2eb-4f8c-bfa5-7053ef20f339
relation.isAuthorOfPublication6da24b6c-7c76-4f3e-9fca-cd68004b9e88
relation.isAuthorOfPublicationd613125b-6f15-4c67-909d-2c1a1157c056
relation.isAuthorOfPublication8ed70b09-b4d3-4a5d-9f75-12b13a332204
relation.isAuthorOfPublication.latestForDiscovery6da24b6c-7c76-4f3e-9fca-cd68004b9e88

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